By ed. by Martin Hiersemann
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Extra info for Activating Unreactive Substrates The Role of Secondary Interactions
Schorm, A. and Sundermeyer, J. (2000) Zeitschrift Fur Anorganische Und Allgemeine Chemie, 626, 1583. , Plackmeyer, J. and Sundermeyer, J. (2001) European Journal of Inorganic Chemistry, 1937. , Saak, W. and Henkel, G. (2000) Journal of The Chemical Society-Dalton Transactions, 3473. , Kipke, J. and Sundermeyer, J. (2001) Inorganic Chemistry, 40, 6964. , Merz, M. and Sundermeyer, J. (2001) Journal of Molecular Catalysis AChemical, 175, 51. , Sundermeyer, J. and Schindler, S. (2004) Angewandte Chemie, 116, 4460; Angewandte Chemie (International Edition in English), (2004) 43, 4360.
9) have never been isolated and structurally characterized. Therefore we follow the concept of generating these intermediates within the sterically demanding ligand regime of these guanidine tripod ligands. 6 Modeling copper-monooxygenase C-H hydroxylation and peroxonitrite formation and decomposition. never been detected, different synthetic routes for their synthesis, namely the reactions of [(TMG3tren)Cu]þ , [(DMEG3tren)Cu]þ and [(HPG3tren)Cu]þ with TsN3, [PhI(NTs)]x and [PhIO]x in MeCN, were chosen.
These reactions can be easily extended to dinuclear or polynuclear complexes as well, but reaction rates in these reactions can be quite different because of the pre-organization of some of the Activating Unreactive Substrates: The Role of Secondary Interactions. Edited by Carsten Bolm and F. Ekkehardt Hahn Copyright Ó 2009 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim ISBN: 978-3-527-31823-0 j 3 Iron Complexes and Dioxygen Activation 40 complexes, thus making their formation much more facile. Furthermore, additional bridging groups can be present and inter- and intramolecular reactions are possible.
Activating Unreactive Substrates The Role of Secondary Interactions by ed. by Martin Hiersemann